Vampire Diaries has been doing a stellar job with music selection lately. A few weeks ago, they chose "I Need To Know" by Kris Allen for a pivotal scene. This week, they used "I Was Wrong" by Sleeperstar (iTunes | Amazon.com) in a big dramatic scene between Damon and Elena where he proclaims his love for her but then makes her forget the moment (HELLO, LET'S STEAL A PLOT LINE FROM ANGEL, OK?!). Great song, though, and it works great with the scene. The song has been climbing up the iTunes charts since the show aired.
Thanks to @Nic_Leigh for bringing the song into my twitter feed yesterday!
Here's the scene: